Carrier dynamics near a crack in GaN microwires with AlGaN multiple quantum wells
Résumé
Relaxation of tensile strain in AlGaN heterostructures grown on GaN template can lead to the formation of
cracks. These extended defects locally degrade the crystal quality resulting in a local increase of non-radiative
recombinations. The effect of such cracks on the optical and structural properties of core-shell AlGaN/AlGaN
multiple quantum wells grown on GaN microwires are comprehensively characterized by means of spectrally
and time-correlated cathodoluminescence (CL). We observe that the CL blueshifts near a crack. By performing
6x6 k.p simulations in combination with transmission electron microscopy analysis, we ascribe this shift to
the strain relaxation by the free surface near cracks. By simultaneously recording the variations of both the
CL lifetime and the CL intensity across the crack, we directly assess the carrier dynamics around the defect
at T = 5 K. We observe that the CL lifetime is reduced typically from 500 ps to less than 300 ps and the CL
intensity increases by about 40% near the crack. The effect of the crack on the optical properties is therefore
of two natures. First, the presence of this defect locally increases non-radiative recombinations while at the
same time, it locally improves the extraction efficiency. These findings emphasize the need for time-resolved
experiments to avoid experimental artifacts related to local changes of light collection
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