Forming ultracold YbAg molecules via photoassociation predicted from ab initio calculations - Archive ouverte HAL
Article Dans Une Revue Physical Review A Année : 2024

Forming ultracold YbAg molecules via photoassociation predicted from ab initio calculations

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This paper discusses the formation of ultracold YbAg molecules via photoassociation, following the proposal of using YbAg as a promising molecular candidate for electron electric dipole moment experiments [M. Verma et al. Phys. Rev. Lett. 125, 153201 (2020)]. Our study utilizes high-level ab initio calculations, encompassing both multireference configuration interaction, relativistic Fock-space coupled cluster, and Kramers-restricted configuration interaction methods, to investigate the electronic structures including potential energy curves, spectroscopic constant, vibrational energy levels, and associated transition dipole moment and Franck-Condon factors for 28 electronic states. By choosing (5)(Ω=3/2) as the intermediate state, we discuss the feasibility of forming ultracold YbAg molecules through stimulated Raman adiabatic passage method.
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hal-04850364 , version 1 (20-12-2024)

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Xiang Yuan, Yong Liu. Forming ultracold YbAg molecules via photoassociation predicted from ab initio calculations. Physical Review A, 2024, 110 (6), pp.062813. ⟨10.1103/PhysRevA.110.062813⟩. ⟨hal-04850364⟩
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