Signatures of a Charge Ice State in the Doped Mott Insulator Nb$_3$Cl$_8$ - Archive ouverte HAL
Pré-Publication, Document De Travail Année : 2024

Signatures of a Charge Ice State in the Doped Mott Insulator Nb$_3$Cl$_8$

Résumé

The interplay between strong electronic correlations and the inherent frustration of certain lattice geometries is a common mechanism for the formation of nontrivial states of matter. In this work, we theoretically explore the collective electronic effects in the monolayer Nb$_3$Cl$_8$, a recently discovered triangular lattice Mott insulator. Our advanced many-body numerical simulations predict the emergence of a phase separation region upon doping this material. Notably, in close proximity to the phase separation, the static charge susceptibility undergoes a drastic change and reveals a distinctive bow-tie structure in momentum space. The appearance of such a signature in the context of spin degrees of freedom would indicate the formation of a spin ice state. This finding allows us to associate the observed phase separation to a charge ice state, a state with a remarkable power-law dependence of both the effective exchange interaction and correlations between electronic densities in real space.
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Dates et versions

hal-04778898 , version 1 (13-11-2024)

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Evgeny Stepanov. Signatures of a Charge Ice State in the Doped Mott Insulator Nb$_3$Cl$_8$. 2024. ⟨hal-04778898⟩
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