Atomic-layer controlled THz Spintronic emission from Epitaxially grown Two dimensional PtSe$_2$/ferromagnet heterostructures - Archive ouverte HAL Accéder directement au contenu
Article Dans Une Revue Advanced Materials Année : 2023

Atomic-layer controlled THz Spintronic emission from Epitaxially grown Two dimensional PtSe$_2$/ferromagnet heterostructures

Martin Mičica
  • Fonction : Auteur
Libor Vojáček
Alain Marty
Jean‐yves Veuillen
  • Fonction : Auteur
Isabelle Gomes de Moraes
  • Fonction : Auteur
Serge Gambarelli
  • Fonction : Auteur
Vincent Maurel
  • Fonction : Auteur
Adrien Wright
  • Fonction : Auteur
Jérôme Tignon
Juliette Mangeney
Jing Li
Frédéric Bonell
Jean‐marie George
  • Fonction : Auteur
Sukhdeep Dhillon
Matthieu Jamet

Résumé

Terahertz (THz) Spintronic emitters based on ferromagnetic/metal junctions have become an important technology for the THz range, offering powerful and ultra-large spectral bandwidths. These developments have driven recent investigations of two-dimensional (2D) materials for new THz spintronic concepts. 2D materials, such as transition metal dichalcogenides (TMDs), are ideal platforms for SCC as they possess strong spin-orbit coupling (SOC) and reduced crystal symmetries. Moreover, SCC and the resulting THz emission can be tuned with the number of layers, electric field or strain. Here, epitaxially grown 1T-PtSe$_2$ and sputtered Ferromagnet (FM) heterostructures are presented as a novel THz emitter where the 1T crystal symmetry and strong SOC favor SCC. High quality of as-grown PtSe$_2$ layers is demonstrated and further FM deposition leaves the PtSe$_2$ unaffected, as evidenced with extensive characterization. Through this atomic growth control, the unique thickness dependent electronic structure of PtSe$_2$ allows the control of the THz emission by SCC. Indeed, we demonstrate the transition from the inverse Rashba-Edelstein effect in one monolayer to the inverse spin Hall effect in multilayers. This band structure flexibility makes PtSe$_2$ an ideal candidate as a THz spintronic 2D material and to explore the underlying mechanisms and engineering of the SCC for THz emission.

Dates et versions

hal-04107294 , version 1 (26-05-2023)

Identifiants

Citer

Khasan Abdukayumov, Martin Mičica, Fatima Ibrahim, Libor Vojáček, Céline Vergnaud, et al.. Atomic-layer controlled THz Spintronic emission from Epitaxially grown Two dimensional PtSe$_2$/ferromagnet heterostructures. Advanced Materials, 2023, pp.2304243. ⟨10.1002/adma.202304243⟩. ⟨hal-04107294⟩
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