Atomic‐Layer Controlled Transition from Inverse Rashba–Edelstein Effect to Inverse Spin Hall Effect in 2D PtSe 2 Probed by THz Spintronic Emission - Archive ouverte HAL Accéder directement au contenu
Article Dans Une Revue Advanced Materials Année : 2024

Atomic‐Layer Controlled Transition from Inverse Rashba–Edelstein Effect to Inverse Spin Hall Effect in 2D PtSe 2 Probed by THz Spintronic Emission

Martin Mičica
  • Fonction : Auteur
Alain Marty
P. Mallet
Adrien Wright
  • Fonction : Auteur
Jérôme Tignon
Juliette Mangeney
Frédéric Bonell
Sukhdeep Dhillon
Matthieu Jamet

Résumé

Abstract 2D materials, such as transition metal dichalcogenides, are ideal platforms for spin‐to‐charge conversion (SCC) as they possess strong spin–orbit coupling (SOC), reduced dimensionality and crystal symmetries as well as tuneable band structure, compared to metallic structures. Moreover, SCC can be tuned with the number of layers, electric field, or strain. Here, SCC in epitaxially grown 2D PtSe 2 by THz spintronic emission is studied since its 1T crystal symmetry and strong SOC favor SCC. High quality of as‐grown PtSe 2 layers is demonstrated, followed by in situ ferromagnet deposition by sputtering that leaves the PtSe 2 unaffected, resulting in well‐defined clean interfaces as evidenced with extensive characterization. Through this atomic growth control and using THz spintronic emission, the unique thickness‐dependent electronic structure of PtSe 2 allows the control of SCC. Indeed, the transition from the inverse Rashba–Edelstein effect (IREE) in 1–3 monolayers (ML) to the inverse spin Hall effect (ISHE) in multilayers (>3 ML) of PtSe 2 enabling the extraction of the perpendicular spin diffusion length and relative strength of IREE and ISHE is demonstrated. This band structure flexibility makes PtSe 2 an ideal candidate to explore the underlying mechanisms and engineering of the SCC as well as for the development of tuneable THz spintronic emitters.

Dates et versions

hal-04107294 , version 1 (26-05-2023)

Identifiants

Citer

Khasan Abdukayumov, Martin Mičica, Fatima Ibrahim, Libor Vojáček, Céline Vergnaud, et al.. Atomic‐Layer Controlled Transition from Inverse Rashba–Edelstein Effect to Inverse Spin Hall Effect in 2D PtSe 2 Probed by THz Spintronic Emission. Advanced Materials, 2024, 36 (14), pp.2304243. ⟨10.1002/adma.202304243⟩. ⟨hal-04107294⟩
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