Electrically-driven insulator-to-metal transition in a correlated insulator: electronic mechanism and thermal description - Archive ouverte HAL
Article Dans Une Revue Physical Review B Année : 2023

Electrically-driven insulator-to-metal transition in a correlated insulator: electronic mechanism and thermal description

Résumé

Motivated by the resistive switchings in transition-metal oxides (TMOs) induced by a voltage bias, we study the far-from-equilibrium dynamics of an electric-field-driven strongly-correlated model featuring a first-order insulator-to-metal transition at equilibrium, namely the dimer-Hubbard model. We use a non-equilibrium implementation of the dynamical cluster approximation to access the steady-state spectral and transport properties. We show that the electric field can drive both metal-to-insulator and insulator-to-metal transitions. While they proceed by quite distinct mechanisms, specifically simple heating of the metal vs. non-equilibrium effects in the correlated charge gap, we show that both these non-equilibrium transitions can be unified in a single framework once the excitations are accounted for in terms of an effective temperature. This conceptual advance brings together the two sides of the long-lasting debate over the origins of the electrically-driven resistive switching in TMOs.

Dates et versions

hal-03876344 , version 1 (28-11-2022)

Identifiants

Citer

Manuel Díaz, Jong Han, Camille Aron. Electrically-driven insulator-to-metal transition in a correlated insulator: electronic mechanism and thermal description. Physical Review B, 2023, 107 (19), pp.195148. ⟨10.1103/PhysRevB.107.195148⟩. ⟨hal-03876344⟩
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