Stress Fluctuations in Glass‐Forming Systems: Elastic Response and Long‐Range Correlations
Résumé
The dynamics of two model glass-formers (3D oligomer melt and 2D polydisperse colloidal system) are analyzed using MD simulations. It is found that the standard deviation of the shear modulus shows a striking peak near the glass transition T g , which is explained with a quantitative theory. The simulation data well below T g suggest that static multi-point correlations of local stress are long-range. The obtained correlation functions of time-dependent and wavevector-resolved stress for the 2D system are in excellent agreement with the developed theory indicating that the frozen-in stress inhomogeneities in the glassy state are correlated according to a power law.
Domaines
Physique [physics]Origine | Fichiers produits par l'(les) auteur(s) |
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