Realization of Polaritonic Topological Charge at Room Temperature Using Polariton Bound States in the Continuum from Perovskite Metasurface
Résumé
Exciton-polaritons are mixed light–matter excitations resulting from the strong coupling regime between an active excitonic material and photonic resonances. Harnessing these hybrid excitations provides a rich playground to explore fascinating fundamental features, as out-of-equilibrium Bose–Einstein condensation and quantum fluids of light, plus novel mechanisms to be exploited in optoelectronic devices. The formation of exciton-polaritons arising from the mixing between hybrid inorganic–organic perovskite excitons and an optical bound state in a continuum (BIC) of a subwavelength-scale metasurface, are experimentally investigated at room temperature. These polaritonic eigenmodes, hereby called polariton BICs (pol-BICs) are revealed in reflectivity, resonant scattering, and photoluminescence measurements. Although pol-BICs only exhibit a finite quality factor bounded by the nonradiative losses of the excitonic component, they fully inherit BIC peculiar features: a full uncoupling from the radiative continuum in the vertical direction, which is associated to a locally vanishing farfield radiation in momentum space. Most importantly, the experimental results confirm that the topological nature of the photonic BIC is perfectly transferred to the pol-BIC. This is evidenced by the observation of a polarization vortex in the farfield of polaritonic emission. The results pave the way to engineer BIC physics of interacting bosons and novel room temperature polaritonic devices
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