Novel approach to nonlinear susceptibility in semiconductors - Archive ouverte HAL
Article Dans Une Revue EPL - Europhysics Letters Année : 2005

Novel approach to nonlinear susceptibility in semiconductors

Résumé

We here propose a new procedure to derive a general expression of the third-order susceptibility valid for any semiconductor Hamiltonian. It relies on our theory for composite exciton many-body effects which is quite appropriate to this problem since all optical nonlinearities in semiconductors come from exchange scatterings with the virtual excitons coupled to photons. Our expression of chi((3)) is sample volume free, as physically expected. It also contains a Pauli term (exchange without Coulomb) which is missed by all bosonized exciton approaches. This term, dominant at large detuning, is a direct manifestation of the exciton composite nature.

Dates et versions

hal-01284405 , version 1 (07-03-2016)

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Monique Combescot, Odile Betbeder-Matibet, K Cho, H Ajiki. Novel approach to nonlinear susceptibility in semiconductors. EPL - Europhysics Letters, 2005, 72 (4), pp.618-623. ⟨10.1209/epl/i2005-10282-0⟩. ⟨hal-01284405⟩
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