Emission characterization of a single CdSe-ZnS nanocrystal with high temporal and spectral resolution by photon-correlation fourier spectroscopy - Archive ouverte HAL
Article Dans Une Revue Physical Review Letters Année : 2008

Emission characterization of a single CdSe-ZnS nanocrystal with high temporal and spectral resolution by photon-correlation fourier spectroscopy

Résumé

We report a spectroscopic study of single colloidal CdSe/ZnS nanocrystals at low temperature. We use photon-correlation Fourier spectroscopy, a technique based on measuring the correlations of the intensities detected at the outputs of a Michelson interferometer. Spectral diffusion over a few mu eV is evidenced, on a typical time scale of 200 mu s. A time resolution as high as 20 mu s is obtained, and an upper limit of 6.5 mu eV emission linewidth is measured, corresponding to a coherence time of at least 200 ps, similar to the values for epitaxial quantum dots.
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hal-01281538 , version 1 (02-03-2016)

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L. Coolen, X. Brokmann, P. Spinicelli, J. -P. Hermier. Emission characterization of a single CdSe-ZnS nanocrystal with high temporal and spectral resolution by photon-correlation fourier spectroscopy. Physical Review Letters, 2008, 100 (2), pp.027403. ⟨10.1103/PhysRevLett.100.027403⟩. ⟨hal-01281538⟩
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