Optimizing Nanoparticle Designs for Ideal Absorption of Light
Résumé
Resonant interaction of light with nanoparticles is essential for a broad range of nanophotonics and
plasmonics applications, including optical antennas, photovoltaics, thermoplasmonics, and sensing. Given this broad
interest, analytical formulas are highly desirable to provide design guidelines for reaching the conditions of ideal
absorption. Here we derive analytical expressions to accurately describe the electric and magnetic modes leading to
ideal absorption. Our model significantly improves on accuracy as compared to classical models using
Green's functions or a Mie coefficient expansion. We demonstrate its applicability over a broad parameter space of
frequencies and particle diameters up to several wavelengths. We reveal that ideal absorption is attainable in
homogeneous spherical nanoparticles made of gold or silver at specific sizes and illumination frequencies. To reach
ideal absorption at virtually any frequency in the visible and near infrared range, we provide explicit guidelines to design
core-shell nanoparticles. This work should prove useful for providing experimental designs that optimize absorption
and for a better understanding of the physics of ideal absorption.
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