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Article Dans Une Revue Journal of Molecular Spectroscopy Année : 2007

CARS methane spectra: Experiments and simulations for temperature diagnostic purposes

Résumé

CARS laboratory experiments were done in the 2905-2925 cm(-1) range, in the vicinity of the v, band of the methane molecule, for pressures ranging from I to 50 bar, and temperatures up to 1100 K. These experiments were carried out in order to retrieve the pressure evolution of the CH4 spectrum, as well as to confirm its temperature dependance. After a brief recall on the theory used to compute pressure broadening coefficients and relaxation rates, we consider the v(3) and v(4) infrared bands of methane for benchmark calculations purposes. Next, we present recent experimental CARS spectra and calculated ones. Lastly, we discuss flame experiments as well as comparisons of temperature retrieval using N-2 and CH4 as probe molecules.

Dates et versions

hal-00400378 , version 1 (30-06-2009)

Identifiants

Citer

Eric Jourdanneau, Tony Gabard, Frédéric Chaussard, R. Saint-Loup, H. Berger, et al.. CARS methane spectra: Experiments and simulations for temperature diagnostic purposes. Journal of Molecular Spectroscopy, 2007, 246, pp.167--179. ⟨10.1016/j.jms.2007.09.006⟩. ⟨hal-00400378⟩
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