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                <term xml:lang="en">Iodine adsorption</term>
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              <p>The nuclear fuel reprocessing industry releases radioactive isotopes into the environmentnotably xenon, krypton and iodine. Among these radionuclides, iodine is highly toxic, mobile andvolatile in the environment. For radioprotection reasons, it is crucial to develop an innovative iodinetrap. As part of the SPECIOSA project, IRSN aims to develop a specific atmospheric samplingdevice for iodine release monitoring into the environment, ensuring the speciation of physicochemical forms (I2 and CH3I). On the one hand, several commercial porous adsorbents (mesoporoussilica, zeolite and activated carbon) were tested for the I2 adsorption in liquid phase. Moreparticularly, silica and zeolites doping with triethylenediamine (TEDA) and copper was achieved toenhance the affinity towards I2 at the expense of CH3I. The obtained adsorption isotherms for I2 inthe liquid phase for these doped materials follow the Langmuir model (Fig.1 A), indicatingtherefore monolayer and homogenous I2 adsorption. Promising performances were also noticedespecially for the TEDA-doped silica material in terms of both adsorption capacities and trappingaffinity. On the other hand, innovative and industrializable MOF formulations are synthesized atUCCS Lille. The obtained powders are shaped by extrusion and spheronization protocols beforefurther tests in gaseous phase (Fig.1 B and C). The extrudates powders were successfully testedwith I2 in the gas phase, showing encouraging performances. The relevant candidates will be testedfor CH3I capture as well as for I2 under more challenging conditions in agreement with the desiredcontext.</p>
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