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                <term xml:lang="en">sea-island structure</term>
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              <p>&lt;div&gt;&lt;p&gt;Polymer dielectrics possessing the superiorities of easy processing and high power density are widely used in pulsed power and power electronics. However, the low energy storage density (U e ) of polymer dielectrics limits their application in the modern electronic industries. In this work, we present the sea-island structure multilayered composites based on Polymethylmethacrylate (PMMA) matrix and Polyvinylidene fluoride (PVDF) nanoparticles, which is constructed by the solution blending with typical solubility differences method and the layer-by-layer solution casting method. The PVDF/PMMA composite incorporated with high PVDF content is placed in the middle of the sandwich-structured composite as a non-traditional intermediate polarization layer. The PVDF/PMMA composite with low PVDF loading is placed in the outer layer to improve the insulating property of the composite. The results show that the PVDF/PMMA composites with inner and outer PVDF volume content of 30 % and 10 %, respectively, obtained an excellent dielectric constant value (ε r ~ 4.35), which is 45 % higher than that of PMMA (ε r ~ 3). Meanwhile, the maximum U e ( ~ 4.95 J cm -3 ) of the PVDF/PMMA composites at an electric field of 422.48 MV m -1 was obtained, which is 207 % higher than that of PMMA (U e ~ 1.61 J cm -3 ). The improved energy storage capability could be attributed to the introduction of highly polarizing particles, the increased number of heterogeneous interfaces, and the multilayered construction of composite. This work provides a strategy for the preparation of advanced all-organic dielectrics with a higher discharge energy density.&lt;/p&gt;&lt;/div&gt;</p>
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