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              <p>Classic viscoelastic systems show correlated storage and loss moduli. To try and decouple them, we study “solid emulsions” witha crosslinked continuous phase. The rheological properties of emulsions depend on both the continuous and the dispersed phase,as well as the interface between them. Thus, by encapsulating the liquid dispersed phase in a solid elastic matrix, we can create acomposite material with tunable rheological properties [1].The chosen dispersed phase in our “solid emulsion” can also solidify at room temperature. This phase change is used to vary themoduli of the dispersed phase. Previous theoretical work has shown that for liquid inclusions we can expect to see differentrheological responses depending on the continuous and dispersed phase moduli, the size of the droplets in the matrix and thevolume fraction of dispersed phase [2, 3]. However, when the inclusions are solid, the complex modulus should only depend onthe continuous phase and volume fraction [4, 5].We first show the feasibility of a composite system whose storage and loss moduli can be controlled independently, and studythe mechanisms for such a decorrelation. For our system, we have observed a decoupling of the storage and loss moduli in therheological response for liquid insertions in the matrix. When the droplets are solid, we observe however a deviation (see Figure1, right) from the expected behavior solely controlled by the matrix and the volume fraction, that we investigate throughrheology and compression-decompression experiments.[1] R. W. Style, R. Tutika, J. Y. Kim, M. D. Bartlett, Advanced Functional Materials, 2020, 31[2] J. F. Palierne, Rheologica Acta, vol. 29, no 3, p. 204‑214, 1990[3] R. Pal, Current Opinion in Colloid &amp;amp; Interface Science, vol. 16, no 1, p. 41‑60, 2011[4] M. Krieger et T. J. Dougherty, Transactions of the Society of Rheology, vol. 3, no 1, p. 137‑152, 1959[5] F. Mahaut et al., Journal of Rheology vol. 52, no 1, pp. 287-313, 2008</p>
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