Improved electro‐actuation property of dielectric elastomer composites regulated by one‐dimensional CaCu 3 Ti 4 O 12 @ TiO 2 core–shell construction - Archive ouverte HAL Accéder directement au contenu
Article Dans Une Revue Journal of Applied Polymer Science Année : 2024

Improved electro‐actuation property of dielectric elastomer composites regulated by one‐dimensional CaCu 3 Ti 4 O 12 @ TiO 2 core–shell construction

Yanfei Gao
  • Fonction : Auteur
Hang Zhao
Na Zhang
  • Fonction : Auteur
Chuying Zhang
  • Fonction : Auteur
Huiqin Wang
  • Fonction : Auteur
Tongguang Zhu
  • Fonction : Auteur

Résumé

Abstract Dielectric elastomers (DEs) are typical electro‐active polymers that can achieve an electro‐actuated deformation under an applied electric field. However, obtaining a large low‐field‐actuated strain of DEs is still a key challenge, which is critical to their practical application range. Herein, a typical CaCu 3 Ti 4 O 12 @TiO 2 (CCTO@TiO 2 ) core–shell‐structured nanowires were synthesized by the micro‐emulsion method. Additionally, a series of polydimethylsiloxane (PDMS)‐based DE composites combining variable proportions of CCTO@TiO 2 were prepared. The CCTO@TiO 2 nanowires with the design of both decreasing dielectric constant from core to shell and a high aspect ratio can provide larger heterogeneous interfaces for the DE composites, leading to a promoted interfacial polarization. The maximum electro‐actuated strain of 37.66% is achieved from the DE composite incorporated with 20 wt% CCTO@TiO 2 when subjected to a relatively low electric field of 40 V/μm, which is 14 times higher than that of pure PDMS (strain ~2.5%). Moreover, the composite exhibits the largest electro‐actuated strain (45.83%) under the electric field approaching its breakdown strength of 43.57 V/μm. The results demonstrate that the one‐dimensional core–shell nanowires have a positive effect on improving the low‐field‐actuated strain of DE composites. This research reveals an effective and feasible method to prepare the DE composites exhibiting enhanced low‐field electro‐actuated characteristics.
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Dates et versions

hal-04479667 , version 1 (27-02-2024)

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Yanfei Gao, Hang Zhao, Na Zhang, Chuying Zhang, Huiqin Wang, et al.. Improved electro‐actuation property of dielectric elastomer composites regulated by one‐dimensional CaCu 3 Ti 4 O 12 @ TiO 2 core–shell construction. Journal of Applied Polymer Science, 2024, ⟨10.1002/app.55379⟩. ⟨hal-04479667⟩
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