Highly dispersed Rh single atoms over graphitic carbon nitride as a robust catalyst for the hydroformylation reaction - Archive ouverte HAL Access content directly
Journal Articles Catalysis Science & Technology Year : 2023

Highly dispersed Rh single atoms over graphitic carbon nitride as a robust catalyst for the hydroformylation reaction

Abstract

Rhodium-catalysed hydroformylation, effective tool in bulk and fine-chemical synthesis, predominantly uses soluble metal complexes. For that reason, the metal leaching and the catalyst recycling are still the major drawbacks of this process. Single-atom catalysts have emerged as a powerful tool to combine the advantages of both homogeneous and heterogeneous catalysts. Since using an appropriate support material is key to create stable, finely dispersed, single-atom catalysts, here we show that Rh atoms anchored on graphitic carbon nitride are robust catalysts for the hydroformylation reaction of styrene.
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hal-04061722 , version 1 (09-06-2023)

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Lole Jurado, Jerome Esvan, Ligia Luque-Álvarez, Luis Bobadilla, José Odriozola, et al.. Highly dispersed Rh single atoms over graphitic carbon nitride as a robust catalyst for the hydroformylation reaction. Catalysis Science & Technology, 2023, 13 (5), pp.1425-1436. ⟨10.1039/D2CY02094G⟩. ⟨hal-04061722⟩
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