Near-critical spreading of droplets - Archive ouverte HAL
Article Dans Une Revue Nature Communications Année : 2022

Near-critical spreading of droplets

Résumé

We study the spreading of droplets in a near-critical phase-separated liquid mixture, using a combination of experiments, lubrication theory and finite-element numerical simulations. The classical Tanner's law describing the spreading of viscous droplets is robustly verified when the critical temperature is neared. Furthermore, the microscopic cut-off length scale emerging in this law is obtained as a single free parameter for each given temperature. In total-wetting conditions, this length is interpreted as the thickness of the thin precursor film present ahead of the apparent contact line. The collapse of the different evolutions onto a single Tanner-like master curve demonstrates the universality of viscous spreading before entering in the fluctuation-dominated regime. Finally, our results reveal a counter-intuitive and sharp thinning of the precursor film when approaching the critical temperature, which is attributed to the vanishing spreading parameter at the critical point.
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Dates et versions

hal-03739843 , version 1 (28-07-2022)
hal-03739843 , version 2 (07-10-2022)

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Raphael Saiseau, Christian Pedersen, Anwar Benjana, Andreas Carlson, Ulysse Delabre, et al.. Near-critical spreading of droplets. Nature Communications, 2022, 13, pp.7442. ⟨hal-03739843v2⟩

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