European aerosol phenomenology − 8: Harmonised source apportionment of organic aerosol using 22 Year-long ACSM/AMS datasets
Gang Chen
(1)
,
Francesco Canonaco
(1, 2)
,
Anna Tobler
(1, 2)
,
Wenche Aas
(3)
,
Andres Alastuey
(4)
,
James Allan
(5)
,
Samira Atabakhsh
(6)
,
Minna Aurela
(7)
,
Urs Baltensperger
(1)
,
Aikaterini Bougiatioti
(8)
,
Joel de Brito
(9)
,
Darius Ceburnis
(10)
,
Benjamin Chazeau
(1, 11)
,
Hasna Chebaicheb
(12, 9)
,
Kaspar Daellenbach
(1)
,
Mikael Ehn
(13)
,
Imad El Haddad
(1)
,
Konstantinos Eleftheriadis
(14)
,
Olivier Favez
(12)
,
Harald Flentje
(15)
,
Anna Font
(16)
,
Kirsten Fossum
(17)
,
Evelyn Freney
(18)
,
Maria Gini
(14)
,
David Green
(16)
,
Liine Heikkinen
(13)
,
Hartmut Herrmann
(6)
,
Athina-Cerise Kalogridis
(14)
,
Hannes Keernik
(19)
,
Radek Lhotka
(20)
,
Chunshui Lin
(17)
,
Chris Lunder
(3)
,
Marek Maasikmets
(21)
,
Manousos Manousakas
(1)
,
Nicolas Marchand
(11)
,
Cristina Marin
(22, 23)
,
Luminita Marmureanu
(22)
,
Nikolaos Mihalopoulos
(8)
,
Griša Močnik
(24, 25)
,
Jaroslaw Nęcki
(26)
,
Colin O'Dowd
(17)
,
Jurgita Ovadnevaite
(17)
,
Thomas Peter
(27)
,
Jean-Eudes Petit
(28)
,
Michael Pikridas
(29)
,
Stephen Matthew Platt
(3)
,
Petra Pokorná
(20)
,
Laurent Poulain
(6)
,
Max Priestman
(16)
,
Véronique Riffault
(9)
,
Matteo Rinaldi
(30)
,
Kazimierz Różański
(31)
,
Jaroslav Schwarz
(20)
,
Jean Sciare
(29)
,
Leïla Simon
(28, 12)
,
Alicja Skiba
(28)
,
Jay Slowik
(1)
,
Yulia Sosedova
(2)
,
Iasonas Stavroulas
(32, 29)
,
Katarzyna Styszko
(26)
,
Erik Teinemaa
(33)
,
Hilkka Timonen
(7)
,
Anja Tremper
(16)
,
Jeni Vasilescu
(22)
,
Marta Via
(34)
,
Petr Vodička
(19)
,
Alfred Wiedensohler
(6)
,
Olga Zografou
(14)
,
María Cruz Minguillón
(34)
,
André S.H. Prévôt
(1)
1
PSI -
Paul Scherrer Institute
2 Datalystica
3 NILU - Norwegian Institute for Air Research
4 CID-CSIC - Centre d'Investigació i Desenvolupament [Barcelona]
5 University of Manchester [Manchester]
6 TROPOS - Leibniz Institute for Tropospheric Research
7 FMI - Finnish Meteorological Institute
8 NOA - National Observatory of Athens
9 CERI EE - IMT Nord Europe - Centre for Energy and Environment
10 Martin Ryan Institute
11 LCE - Laboratoire Chimie de l'environnement
12 INERIS - Institut National de l'Environnement Industriel et des Risques
13 INAR - Institute for Atmospheric and Earth System Research
14 NCSR - National Center for Scientific Research "Demokritos"
15 MOHp - Meteorologisches Observatorium Hohenpeißenberg
16 Imperial College London
17 NUI Galway - National University of Ireland [Galway]
18 LaMP - Laboratoire de Météorologie Physique
19 TTÜ - Tallinn University of Technology
20 CAS - Czech Academy of Sciences [Prague]
21 Estonian Environmental Research Center, Tallinn, Estonia
22 INOE - National Institute of Research and Development for Optoelectronics
23 UPB - University Politehnica of Bucharest [Romania]
24 IJS - Jozef Stefan Institute [Ljubljana]
25 University of Nova Gorica
26 AGH UST - AGH University of Science and Technology [Krakow, PL]
27 D-USYS - Department of Environmental Systems Science [ETH Zürich]
28 LSCE - Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette]
29 Climate and Atmosphere Research Centre (CARE-C), The Cyprus Institute, Nicosia, 2121, Cyprus
30 ISAC - Istituto di Scienze dell'Atmosfera e del Clima [Bologna]
31 FPACS - Faculty of Physics and Applied Computer Science [Kraków]
32 AMU - Aix Marseille Université
33 EKUK - Estonian Environmental Research Centre
34 CSIC - Consejo Superior de Investigaciones Científicas [Spain]
2 Datalystica
3 NILU - Norwegian Institute for Air Research
4 CID-CSIC - Centre d'Investigació i Desenvolupament [Barcelona]
5 University of Manchester [Manchester]
6 TROPOS - Leibniz Institute for Tropospheric Research
7 FMI - Finnish Meteorological Institute
8 NOA - National Observatory of Athens
9 CERI EE - IMT Nord Europe - Centre for Energy and Environment
10 Martin Ryan Institute
11 LCE - Laboratoire Chimie de l'environnement
12 INERIS - Institut National de l'Environnement Industriel et des Risques
13 INAR - Institute for Atmospheric and Earth System Research
14 NCSR - National Center for Scientific Research "Demokritos"
15 MOHp - Meteorologisches Observatorium Hohenpeißenberg
16 Imperial College London
17 NUI Galway - National University of Ireland [Galway]
18 LaMP - Laboratoire de Météorologie Physique
19 TTÜ - Tallinn University of Technology
20 CAS - Czech Academy of Sciences [Prague]
21 Estonian Environmental Research Center, Tallinn, Estonia
22 INOE - National Institute of Research and Development for Optoelectronics
23 UPB - University Politehnica of Bucharest [Romania]
24 IJS - Jozef Stefan Institute [Ljubljana]
25 University of Nova Gorica
26 AGH UST - AGH University of Science and Technology [Krakow, PL]
27 D-USYS - Department of Environmental Systems Science [ETH Zürich]
28 LSCE - Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette]
29 Climate and Atmosphere Research Centre (CARE-C), The Cyprus Institute, Nicosia, 2121, Cyprus
30 ISAC - Istituto di Scienze dell'Atmosfera e del Clima [Bologna]
31 FPACS - Faculty of Physics and Applied Computer Science [Kraków]
32 AMU - Aix Marseille Université
33 EKUK - Estonian Environmental Research Centre
34 CSIC - Consejo Superior de Investigaciones Científicas [Spain]
Joel de Brito
- Fonction : Auteur
- PersonId : 20128
- IdHAL : joel-ferreira-de-brito
- ORCID : 0000-0002-4420-9442
- IdRef : 253123364
Olivier Favez
- Fonction : Auteur
- PersonId : 1090231
- IdHAL : olivier-favez
- ORCID : 0000-0002-8821-1923
Anna Font
- Fonction : Auteur
- PersonId : 1281423
- IdHAL : anna-font
- ORCID : 0000-0003-1488-8090
Nicolas Marchand
- Fonction : Auteur
- PersonId : 12297
- IdHAL : n-marchand
- ORCID : 0000-0001-9745-492X
- IdRef : 073960608
Véronique Riffault
- Fonction : Auteur
- PersonId : 856
- IdHAL : veronique-riffault
- ORCID : 0000-0001-5572-0871
- IdRef : 070462992
María Cruz Minguillón
- Fonction : Auteur correspondant
Résumé
Organic aerosol (OA) is a key component of total submicron particulate matter (PM1), and comprehensive
knowledge of OA sources across Europe is crucial to mitigate PM1 levels. Europe has a well-established air quality
research infrastructure from which yearlong datasets using 21 aerosol chemical speciation monitors (ACSMs) and
1 aerosol mass spectrometer (AMS) were gathered during 2013–2019. It includes 9 non-urban and 13 urban sites.
This study developed a state-of-the-art source apportionment protocol to analyse long-term OA mass spectrum
data by applying the most advanced source apportionment strategies (i.e., rolling PMF, ME-2, and bootstrap).
This harmonised protocol was followed strictly for all 22 datasets, making the source apportionment results more
comparable. In addition, it enables quantification of the most common OA components such as hydrocarbon-like
OA (HOA), biomass burning OA (BBOA), cooking-like OA (COA), more oxidised-oxygenated OA (MO-OOA), and
less oxidised-oxygenated OA (LO-OOA). Other components such as coal combustion OA (CCOA), solid fuel OA
(SFOA: mainly mixture of coal and peat combustion), cigarette smoke OA (CSOA), sea salt (mostly inorganic but
part of the OA mass spectrum), coffee OA, and ship industry OA could also be separated at a few specific sites.
Oxygenated OA (OOA) components make up most of the submicron OA mass (average = 71.1%, range from 43.7
to 100%). Solid fuel combustion-related OA components (i.e., BBOA, CCOA, and SFOA) are still considerable
with in total 16.0% yearly contribution to the OA, yet mainly during winter months (21.4%). Overall, this
comprehensive protocol works effectively across all sites governed by different sources and generates robust and
consistent source apportionment results. Our work presents a comprehensive overview of OA sources in Europe
with a unique combination of high time resolution (30–240 min) and long-term data coverage (9–36 months),
providing essential information to improve/validate air quality, health impact, and climate models.
Format du dépôt | Fichier |
---|---|
Type de dépôt | Article dans une revue |
Titre |
en
European aerosol phenomenology − 8: Harmonised source apportionment of organic aerosol using 22 Year-long ACSM/AMS datasets
|
Résumé |
en
Organic aerosol (OA) is a key component of total submicron particulate matter (PM1), and comprehensive
knowledge of OA sources across Europe is crucial to mitigate PM1 levels. Europe has a well-established air quality
research infrastructure from which yearlong datasets using 21 aerosol chemical speciation monitors (ACSMs) and
1 aerosol mass spectrometer (AMS) were gathered during 2013–2019. It includes 9 non-urban and 13 urban sites.
This study developed a state-of-the-art source apportionment protocol to analyse long-term OA mass spectrum
data by applying the most advanced source apportionment strategies (i.e., rolling PMF, ME-2, and bootstrap).
This harmonised protocol was followed strictly for all 22 datasets, making the source apportionment results more
comparable. In addition, it enables quantification of the most common OA components such as hydrocarbon-like
OA (HOA), biomass burning OA (BBOA), cooking-like OA (COA), more oxidised-oxygenated OA (MO-OOA), and
less oxidised-oxygenated OA (LO-OOA). Other components such as coal combustion OA (CCOA), solid fuel OA
(SFOA: mainly mixture of coal and peat combustion), cigarette smoke OA (CSOA), sea salt (mostly inorganic but
part of the OA mass spectrum), coffee OA, and ship industry OA could also be separated at a few specific sites.
Oxygenated OA (OOA) components make up most of the submicron OA mass (average = 71.1%, range from 43.7
to 100%). Solid fuel combustion-related OA components (i.e., BBOA, CCOA, and SFOA) are still considerable
with in total 16.0% yearly contribution to the OA, yet mainly during winter months (21.4%). Overall, this
comprehensive protocol works effectively across all sites governed by different sources and generates robust and
consistent source apportionment results. Our work presents a comprehensive overview of OA sources in Europe
with a unique combination of high time resolution (30–240 min) and long-term data coverage (9–36 months),
providing essential information to improve/validate air quality, health impact, and climate models.
|
Auteur(s) |
Gang Chen
1
, Francesco Canonaco
1, 2
, Anna Tobler
1, 2
, Wenche Aas
3
, Andres Alastuey
4
, James Allan
5
, Samira Atabakhsh
6
, Minna Aurela
7
, Urs Baltensperger
1
, Aikaterini Bougiatioti
8
, Joel de Brito
9
, Darius Ceburnis
10
, Benjamin Chazeau
1, 11
, Hasna Chebaicheb
12, 9
, Kaspar Daellenbach
1
, Mikael Ehn
13
, Imad El Haddad
1
, Konstantinos Eleftheriadis
14
, Olivier Favez
12
, Harald Flentje
15
, Anna Font
16
, Kirsten Fossum
17
, Evelyn Freney
18
, Maria Gini
14
, David Green
16
, Liine Heikkinen
13
, Hartmut Herrmann
6
, Athina-Cerise Kalogridis
14
, Hannes Keernik
19
, Radek Lhotka
20
, Chunshui Lin
17
, Chris Lunder
3
, Marek Maasikmets
21
, Manousos Manousakas
1
, Nicolas Marchand
11
, Cristina Marin
22, 23
, Luminita Marmureanu
22
, Nikolaos Mihalopoulos
8
, Griša Močnik
24, 25
, Jaroslaw Nęcki
26
, Colin O'Dowd
17
, Jurgita Ovadnevaite
17
, Thomas Peter
27
, Jean-Eudes Petit
28
, Michael Pikridas
29
, Stephen Matthew Platt
3
, Petra Pokorná
20
, Laurent Poulain
6
, Max Priestman
16
, Véronique Riffault
9
, Matteo Rinaldi
30
, Kazimierz Różański
31
, Jaroslav Schwarz
20
, Jean Sciare
29
, Leïla Simon
28, 12
, Alicja Skiba
28
, Jay Slowik
1
, Yulia Sosedova
2
, Iasonas Stavroulas
32, 29
, Katarzyna Styszko
26
, Erik Teinemaa
33
, Hilkka Timonen
7
, Anja Tremper
16
, Jeni Vasilescu
22
, Marta Via
34
, Petr Vodička
19
, Alfred Wiedensohler
6
, Olga Zografou
14
, María Cruz Minguillón
34
, André S.H. Prévôt
1
1
PSI -
Paul Scherrer Institute
( 1961 )
- Villigen PSI, CH5232 Villigen, Suisse
- Suisse
2
Datalystica
( 1095569 )
- Suisse
3
NILU -
Norwegian Institute for Air Research
( 483134 )
- Instituttveien 18, 2007 Kjeller
- Norvège
4
CID-CSIC -
Centre d'Investigació i Desenvolupament [Barcelona]
( 1066081 )
- C. Jordi Girona, 18-26. Barcelona. E-08034
- Espagne
5
University of Manchester [Manchester]
( 121172 )
- Oxford Rd, Manchester M13 9PL
- Royaume-Uni
6
TROPOS -
Leibniz Institute for Tropospheric Research
( 480247 )
- Permoserstrasse 15, 04318 Leipzig
- Allemagne
7
FMI -
Finnish Meteorological Institute
( 480531 )
- Erik Palmenin aukio 1, P.O. Box 503, 00 101 Helsinki, Finland
- Finlande
8
NOA -
National Observatory of Athens
( 313251 )
- Lofos Nymphon - Thissio, PO Box 20048 - 11810, Athens
- Grèce
9
CERI EE - IMT Nord Europe -
Centre for Energy and Environment
( 1076754 )
- Cité Scientifique, Rue Guglielmo Marconi BP 20145 VILLENEUVE D’ASCQ
- France
10
Martin Ryan Institute
( 435064 )
- Irlande
11
LCE -
Laboratoire Chimie de l'environnement
( 220811 )
- Case 29
3 place Victor Hugo
13331 Marseille Cedex 3
- France
12
INERIS -
Institut National de l'Environnement Industriel et des Risques
( 3186 )
- Verneuil-en-Halatte ; Nancy ; Aix en Provence
- France
13
INAR -
Institute for Atmospheric and Earth System Research
( 1039416 )
- P.O. BOx 64, 00014 Helsinki
- Finlande
14
NCSR -
National Center for Scientific Research "Demokritos"
( 139275 )
- Agia Paraskevi Attikis, P.O.Box 60228, 153 10 ATHENS, GREECE
- Grèce
15
MOHp -
Meteorologisches Observatorium Hohenpeißenberg
( 451326 )
- Albin-Schwaiger-Weg 10, 82383 Hohenpeissenberg
- Allemagne
16
Imperial College London
( 69530 )
- South Kensington Campus, London SW7 2AZ
- Royaume-Uni
17
NUI Galway -
National University of Ireland [Galway]
( 373032 )
- Irlande
18
LaMP -
Laboratoire de Météorologie Physique
( 1063673 )
- 4 avenue Blaise Pascal, TSA 60026 / CS 60026, 63178 Aubière Cedex
- France
19
TTÜ -
Tallinn University of Technology
( 310135 )
- Ehitajate tee 5, 19086 Tallinn
- Estonie
20
CAS -
Czech Academy of Sciences [Prague]
( 311871 )
- Národní 3, 117 20 Prague 1
- Tchéquie
21
Estonian Environmental Research Center, Tallinn, Estonia
( 562685 )
- Estonie
22
INOE -
National Institute of Research and Development for Optoelectronics
( 409353 )
- Magurele, 77125, Romania
- Roumanie
23
UPB -
University Politehnica of Bucharest [Romania]
( 204332 )
- Splaiul Independentei nr. 313, sector 6, Bucuresti
CP 060042
ROUMANIE
- Roumanie
24
IJS -
Jozef Stefan Institute [Ljubljana]
( 451147 )
- Jamova cesta 39, 1000 Ljubljana Slovenia
- Slovénie
25
University of Nova Gorica
( 41110 )
- Vipavska 13, 5000 Nova Gorica
- Slovénie
26
AGH UST -
AGH University of Science and Technology [Krakow, PL]
( 445585 )
- al. Mickiewicza 30,
30-059 Krakow,
Poland
- Pologne
27
D-USYS -
Department of Environmental Systems Science [ETH Zürich]
( 497712 )
- Universitätstrasse 2, CH-8092 Zürich
- Suisse
28
LSCE -
Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette]
( 518 )
- Bât. 12,
avenue de la Terrasse,
F-91198 GIF-SUR-YVETTE CEDEX
- France
29
Climate and Atmosphere Research Centre (CARE-C), The Cyprus Institute, Nicosia, 2121, Cyprus
( 1075040 )
- Chypre
30
ISAC -
Istituto di Scienze dell'Atmosfera e del Clima [Bologna]
( 543831 )
- Via P. Gobetti 101, 40129 Bologna
- Italie
31
FPACS -
Faculty of Physics and Applied Computer Science [Kraków]
( 489850 )
- Pologne
32
AMU -
Aix Marseille Université
( 198056 )
- Aix-Marseille Université
Jardins du Pharo
58 Boulevard Charles Livon
13284 Marseille cedex 7
- France
33
EKUK -
Estonian Environmental Research Centre
( 1050917 )
- Marja 4d, 10617 Tallinn
- Estonie
34
CSIC -
Consejo Superior de Investigaciones Científicas [Spain]
( 1001769 )
- Séville
- Espagne
|
URL éditeur |
https://www.sciencedirect.com/science/article/pii/S0160412022002525?via%3Dihub
|
Date de publication |
2022-08
|
Licence |
Paternité
|
Langue du document |
Anglais
|
Nom de la revue |
|
Vulgarisation |
Non
|
Comité de lecture |
Oui
|
Audience |
Internationale
|
Volume |
166
|
Page/Identifiant |
107325
|
Projet(s) Européen(s) |
|
Projet(s) ANR |
|
Domaine(s) |
|
Financement |
|
arXiv Id | 2201.00579 |
DOI | 10.1016/j.envint.2022.107325 |
Origine :
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