Unveiling the coupling of single metallic nanoparticles to whispering-gallery microcavities - Archive ouverte HAL
Article Dans Une Revue Nano Letters Année : 2021

Unveiling the coupling of single metallic nanoparticles to whispering-gallery microcavities

Résumé

Whispering gallery mode resonators (WGMRs) trap light over many optical periods using total internal reflection. Thereby, they host multiple narrowband circulating modes that find applications in quantum electrodynamics, optomechanics, sensing and lasing. The spherical symmetry and low field leakage of dielectric microspheres make it difficult to probe their high-quality optical modes using far-field radiation. However, local field enhancement from metallic nanoparticles (MNPs) placed at the edge of the resonators can interface the optical far-field and the bounded cavity modes. In this work, we study the interaction between whispering gallery modes and the MNP surface plasmons with nanometric spatial resolution by using electron-beam spectroscopies in a scanning transmission electron microscope. We show that gallery modes are induced over the spectral range of the dipolar plasmons of the nanoparticle. Additionally, we explore the dependence of the transverse electric and transverse magnetic polarization of the induced gallery mode on the induced dipole moment of the MNP. Our study demonstrates a viable mechanism to effectively excite high-quality-factor whispering gallery modes and holds potential for applications in optical sensing and light manipulation.

Dates et versions

hal-03373950 , version 1 (11-10-2021)

Identifiants

Citer

Yves Auad, Cyrille Hamon, Marcel Tencé, Hugo Lourenço-Martins, Vahagn Mkhitaryan, et al.. Unveiling the coupling of single metallic nanoparticles to whispering-gallery microcavities. Nano Letters, 2021, ⟨10.1021/acs.nanolett.1c03826⟩. ⟨hal-03373950⟩
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