Observation of Ultrafast Self-Action Effects in Quasi-BIC Resonant Metasurfaces - Archive ouverte HAL
Article Dans Une Revue Nano Letters Année : 2021

Observation of Ultrafast Self-Action Effects in Quasi-BIC Resonant Metasurfaces

Ivan Sinev
Kirill Koshelev
Zhuojun Liu
  • Fonction : Auteur
Anton Rudenko
Konstantin Ladutenko
  • Fonction : Auteur
Alexey Shcherbakov
Zarina Sadrieva
  • Fonction : Auteur
Mikhail Baranov
  • Fonction : Auteur
Tatiana Itina
Jin Liu
Andrey Bogdanov
Yuri Kivshar
  • Fonction : Auteur
  • PersonId : 1097722

Résumé

High-index dielectric metasurfaces can support sharp optical resonances enabled by the physics of bound states in the continuum (BICs) often manifested in experiments as quasi-BIC resonances. They provide a way to enhance light–matter interaction at the subwavelength scale bringing novel opportunities for nonlinear nanophotonics. Strong narrow-band field enhancement in quasi-BIC metasurfaces leads to an extreme sensitivity to a change of the refractive index that may limit nonlinear functionalities for the pump intensities beyond the perturbative regime. Here we study ultrafast self-action effects observed in quasi-BIC silicon metasurfaces and demonstrate how they alter the power dependence of the third-harmonic generation efficiency. We study experimentally a transition from the subcubic to supercubic regimes for the generated third-harmonic power driven by a blue-shift of the quasi-BIC in the multiphoton absorption regime. Our results suggest a way to implement ultrafast nonlinear dynamics in high-index resonant dielectric metasurfaces for nonlinear meta-optics beyond the perturbative regime.
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Dates et versions

hal-03352301 , version 1 (23-09-2021)

Identifiants

Citer

Ivan Sinev, Kirill Koshelev, Zhuojun Liu, Anton Rudenko, Konstantin Ladutenko, et al.. Observation of Ultrafast Self-Action Effects in Quasi-BIC Resonant Metasurfaces. Nano Letters, inPress, 21 (20), pp.8848-8855. ⟨10.1021/acs.nanolett.1c03257⟩. ⟨hal-03352301⟩
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