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            <funder>Financial support from Aix-Marseille Université, the Centre National de la Recherche Scientifique (CNRS), and Centrale Marseille is gratefully acknowledged. P.L. thanks the China Scholarship Council (No. 201701810027) for support. This work was supported by the computing facilities of the CRCMM, “Centre Régional de Compé tences en Modélisation Moléculaire de Marseille”.</funder>
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                <term xml:lang="en">enantioselective organocatalysis</term>
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              <p>An expedient synthesis of a new family of configurationally stable dioxa[6]helicenes was established using a sequential helicoselective organocatalyzed heteroannulation/eliminative aromatization via enantioenriched fused 2-nitro dihydrofurans featuring both central and helical chiralities. Starting from simple achiral precursors, a broad range of these previously unknown chiral heterocyclic scaffolds were obtained with good efficiency, and their aromatization proceeded with very high enantiopurity retention in most cases.</p>
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