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              <p>We combined a spin resolved photoemission spectrometer with a high-harmonic generation (HHG) lasersource in order to perform spin, time, and angle resolved photoemission spectroscopy (STARPES) experimentson the transition metal dichalcogenide bulk WTe2, a possible Weyl type-II semimetal. Measurements at differentfemtosecond pump-probe delays and comparison with spin resolved one-step photoemission calculations provideinsight into the spin polarization of electrons above the Fermi level in the region where Weyl points of WTe2 areexpected. We observe a spin accumulation above the Weyl points region, which is consistent with a spin-selectivebottleneck effect due to the presence of spin-polarized conelike electronic structure. Our results support thefeasibility of STARPES with HHG, which despite being experimentally challenging provides a unique way tostudy spin dynamics in photoemission.</p>
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