A dicopper( i )-dimesoionic carbene complex as a click catalyst: mechanistic implications - Archive ouverte HAL
Article Dans Une Revue Dalton Transactions Année : 2019

A dicopper( i )-dimesoionic carbene complex as a click catalyst: mechanistic implications

Résumé

A dicopper(I) complex comprising a dimesoionic carbene and an acetate-bridge is synthesized and fully characterized. This complex is a potent pre-catalyst for the azide–alkyne cycloaddition reaction. A full kinetic investigation shows a first order in azide and a catalyst order smaller than one due to an equilibrated dimerization of the catalyst.

Domaines

Chimie
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Dates et versions

hal-02194919 , version 1 (26-07-2019)

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Citer

Julia Beerhues, Kévin Fauché, Federico Cisnetti, Biprajit Sarkar, Arnaud Gautier. A dicopper( i )-dimesoionic carbene complex as a click catalyst: mechanistic implications. Dalton Transactions, 2019, 48 (24), pp.8931-8936. ⟨10.1039/C9DT01882D⟩. ⟨hal-02194919⟩
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