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            <title xml:lang="en">Diurnal Variability of Persistent Organic Pollutants in the Atmosphere over the Remote Southern Atlantic Ocean</title>
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                <forename type="first">Rosalinda</forename>
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                <title xml:lang="en">Diurnal Variability of Persistent Organic Pollutants in the Atmosphere over the Remote Southern Atlantic Ocean</title>
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              <p>A diel (24-h) cycle with daytime atmospheric concentrations higher thannighttime concentrations by a factor of 1.5–3 was observed for several low molecularweight polychlorinated biphenyls (PCBs) and polycyclic aromatic hydrocarbons (PAHs) inremote areas of the tropical South Atlantic during a cruise in October–November 2005. Incontrast, high molecular weight PCBs and PAHs did not display diurnal variability. Amodel which has successfully explained diel variability of persistent organic pollutants (POPs)over land could not reproduce the observed diel cycle by considering variability intemperature, atmospheric OH radical concentrations, atmospheric boundary layer heightand wind speed as causal factors. We used the model to conduct two bounding scenarios toexplore the possibility that phytoplankton biomass turn-over in the surface ocean drives theobserved variability in air concentrations. The model could only qualitatively reproduce thefield observations of diel variability for low chlorinated PCB congeners when the oceanacts as a source of pollutants to the atmosphere, and when variability in biomass drivesvariability in the capacity of the surface ocean.</p>
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