<?xml version="1.0" encoding="utf-8"?>
<TEI xmlns="http://www.tei-c.org/ns/1.0" xmlns:xsi="http://www.w3.org/2001/XMLSchema-instance" xmlns:hal="http://hal.archives-ouvertes.fr/" xmlns:gml="http://www.opengis.net/gml/3.3/" xmlns:gmlce="http://www.opengis.net/gml/3.3/ce" version="1.1" xsi:schemaLocation="http://www.tei-c.org/ns/1.0 http://api.archives-ouvertes.fr/documents/aofr-sword.xsd">
  <teiHeader>
    <fileDesc>
      <titleStmt>
        <title>HAL TEI export of hal-01963243</title>
      </titleStmt>
      <publicationStmt>
        <distributor>CCSD</distributor>
        <availability status="restricted">
          <licence target="https://creativecommons.org/publicdomain/zero/1.0/">CC0 1.0 - Universal</licence>
        </availability>
        <date when="2026-05-16T01:43:13+02:00"/>
      </publicationStmt>
      <sourceDesc>
        <p part="N">HAL API Platform</p>
      </sourceDesc>
    </fileDesc>
  </teiHeader>
  <text>
    <body>
      <listBibl>
        <biblFull>
          <titleStmt>
            <title xml:lang="en">Interface disorder in large single- and multi-shell upconverting nanocrystals</title>
            <author role="aut">
              <persName>
                <forename type="first">Damien</forename>
                <surname>Hudry</surname>
              </persName>
              <idno type="halauthorid">1488253-0</idno>
              <affiliation ref="#struct-150665"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Radian</forename>
                <surname>Popescu</surname>
              </persName>
              <idno type="halauthorid">1488254-0</idno>
              <affiliation ref="#struct-150665"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Dmitry</forename>
                <surname>Busko</surname>
              </persName>
              <idno type="halauthorid">1488255-0</idno>
              <affiliation ref="#struct-150665"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Maria</forename>
                <surname>Diaz-Lopez</surname>
              </persName>
              <idno type="halauthorid">1410133-0</idno>
              <affiliation ref="#struct-1042408"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Milinda</forename>
                <surname>Abeykoon</surname>
              </persName>
              <idno type="halauthorid">1488256-0</idno>
              <affiliation ref="#struct-3392"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Pierre</forename>
                <surname>Bordet</surname>
              </persName>
              <email type="md5">a4df6b31a083716d8a6aee1d1618536b</email>
              <email type="domain">neel.cnrs.fr</email>
              <idno type="idhal" notation="string">pierre-bordet</idno>
              <idno type="idhal" notation="numeric">5625</idno>
              <idno type="halauthorid" notation="string">19706-5625</idno>
              <idno type="RESEARCHERID">http://www.researcherid.com/rid/A-6077-2016</idno>
              <idno type="ORCID">https://orcid.org/0000-0002-1488-2257</idno>
              <idno type="IDREF">https://www.idref.fr/060598921</idno>
              <idno type="RESEARCHERID">http://www.researcherid.com/rid/http://www.researcherid.com/rid/A-6077-2016</idno>
              <affiliation ref="#struct-1042408"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Dagmar</forename>
                <surname>Gerthsen</surname>
              </persName>
              <idno type="halauthorid">1488257-0</idno>
              <affiliation ref="#struct-150665"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Ian</forename>
                <surname>Howard</surname>
              </persName>
              <idno type="halauthorid">1074608-0</idno>
              <affiliation ref="#struct-150665"/>
            </author>
            <author role="aut">
              <persName>
                <forename type="first">Bryce</forename>
                <surname>Richards</surname>
              </persName>
              <idno type="halauthorid">1488258-0</idno>
              <affiliation ref="#struct-150665"/>
            </author>
            <editor role="depositor">
              <persName>
                <forename>Pierre</forename>
                <surname>Bordet</surname>
              </persName>
              <email type="md5">a4df6b31a083716d8a6aee1d1618536b</email>
              <email type="domain">neel.cnrs.fr</email>
            </editor>
          </titleStmt>
          <editionStmt>
            <edition n="v1" type="current">
              <date type="whenSubmitted">2024-12-02 09:15:40</date>
              <date type="whenModified">2026-04-13 14:24:02</date>
              <date type="whenReleased">2024-12-05 11:20:53</date>
              <date type="whenProduced">2019</date>
              <date type="whenEndEmbargoed">2024-12-02</date>
              <ref type="file" target="https://hal.science/hal-01963243v1/document">
                <date notBefore="2024-12-02"/>
              </ref>
              <ref type="file" subtype="author" n="1" target="https://hal.science/hal-01963243v1/file/b600a7aa9a9e8b0bdd77a5d85b6b2b0d.pdf" id="file-4813545-4198956">
                <date notBefore="2024-12-02"/>
              </ref>
              <ref type="externalLink" target="https://www.osti.gov/biblio/1502807"/>
            </edition>
            <respStmt>
              <resp>contributor</resp>
              <name key="116496">
                <persName>
                  <forename>Pierre</forename>
                  <surname>Bordet</surname>
                </persName>
                <email type="md5">a4df6b31a083716d8a6aee1d1618536b</email>
                <email type="domain">neel.cnrs.fr</email>
              </name>
            </respStmt>
          </editionStmt>
          <publicationStmt>
            <distributor>CCSD</distributor>
            <idno type="halId">hal-01963243</idno>
            <idno type="halUri">https://hal.science/hal-01963243</idno>
            <idno type="halBibtex">hudry:hal-01963243</idno>
            <idno type="halRefHtml">&lt;i&gt;Journal of Materials Chemistry C&lt;/i&gt;, 2019, 7 (5), pp.1164-1172. &lt;a target="_blank" href="https://dx.doi.org/10.1039/C8TC05130E"&gt;&amp;#x27E8;10.1039/C8TC05130E&amp;#x27E9;&lt;/a&gt;</idno>
            <idno type="halRef">Journal of Materials Chemistry C, 2019, 7 (5), pp.1164-1172. &amp;#x27E8;10.1039/C8TC05130E&amp;#x27E9;</idno>
            <availability status="restricted">
              <licence target="https://about.hal.science/hal-authorisation-v1/">HAL Authorization<ref corresp="#file-4813545-4198956"/></licence>
            </availability>
          </publicationStmt>
          <seriesStmt>
            <idno type="stamp" n="UGA">HAL Grenoble Alpes</idno>
            <idno type="stamp" n="CNRS">CNRS - Centre national de la recherche scientifique</idno>
            <idno type="stamp" n="INPG">Institut polytechnique de Grenoble</idno>
            <idno type="stamp" n="NEEL">Institut Néel</idno>
            <idno type="stamp" n="NEEL-MRS">Matériaux, rayonnements, structure</idno>
            <idno type="stamp" n="UGA-COMUE">Université Grenoble Alpes [2016-2019]</idno>
            <idno type="stamp" n="TEST-UGA">TEST-UGA</idno>
          </seriesStmt>
          <notesStmt>
            <note type="audience" n="2">International</note>
            <note type="popular" n="0">No</note>
            <note type="peer" n="1">Yes</note>
          </notesStmt>
          <sourceDesc>
            <biblStruct>
              <analytic>
                <title xml:lang="en">Interface disorder in large single- and multi-shell upconverting nanocrystals</title>
                <author role="aut">
                  <persName>
                    <forename type="first">Damien</forename>
                    <surname>Hudry</surname>
                  </persName>
                  <idno type="halauthorid">1488253-0</idno>
                  <affiliation ref="#struct-150665"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Radian</forename>
                    <surname>Popescu</surname>
                  </persName>
                  <idno type="halauthorid">1488254-0</idno>
                  <affiliation ref="#struct-150665"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Dmitry</forename>
                    <surname>Busko</surname>
                  </persName>
                  <idno type="halauthorid">1488255-0</idno>
                  <affiliation ref="#struct-150665"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Maria</forename>
                    <surname>Diaz-Lopez</surname>
                  </persName>
                  <idno type="halauthorid">1410133-0</idno>
                  <affiliation ref="#struct-1042408"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Milinda</forename>
                    <surname>Abeykoon</surname>
                  </persName>
                  <idno type="halauthorid">1488256-0</idno>
                  <affiliation ref="#struct-3392"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Pierre</forename>
                    <surname>Bordet</surname>
                  </persName>
                  <email type="md5">a4df6b31a083716d8a6aee1d1618536b</email>
                  <email type="domain">neel.cnrs.fr</email>
                  <idno type="idhal" notation="string">pierre-bordet</idno>
                  <idno type="idhal" notation="numeric">5625</idno>
                  <idno type="halauthorid" notation="string">19706-5625</idno>
                  <idno type="RESEARCHERID">http://www.researcherid.com/rid/A-6077-2016</idno>
                  <idno type="ORCID">https://orcid.org/0000-0002-1488-2257</idno>
                  <idno type="IDREF">https://www.idref.fr/060598921</idno>
                  <idno type="RESEARCHERID">http://www.researcherid.com/rid/http://www.researcherid.com/rid/A-6077-2016</idno>
                  <affiliation ref="#struct-1042408"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Dagmar</forename>
                    <surname>Gerthsen</surname>
                  </persName>
                  <idno type="halauthorid">1488257-0</idno>
                  <affiliation ref="#struct-150665"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Ian</forename>
                    <surname>Howard</surname>
                  </persName>
                  <idno type="halauthorid">1074608-0</idno>
                  <affiliation ref="#struct-150665"/>
                </author>
                <author role="aut">
                  <persName>
                    <forename type="first">Bryce</forename>
                    <surname>Richards</surname>
                  </persName>
                  <idno type="halauthorid">1488258-0</idno>
                  <affiliation ref="#struct-150665"/>
                </author>
              </analytic>
              <monogr>
                <idno type="halJournalId" status="VALID">102239</idno>
                <idno type="issn">2050-7526</idno>
                <idno type="eissn">2050-7534</idno>
                <title level="j">Journal of Materials Chemistry C</title>
                <imprint>
                  <publisher>Royal Society of Chemistry</publisher>
                  <biblScope unit="volume">7</biblScope>
                  <biblScope unit="issue">5</biblScope>
                  <biblScope unit="pp">1164-1172</biblScope>
                  <date type="datePub">2019</date>
                </imprint>
              </monogr>
              <idno type="doi">10.1039/C8TC05130E</idno>
            </biblStruct>
          </sourceDesc>
          <profileDesc>
            <langUsage>
              <language ident="en">English</language>
            </langUsage>
            <textClass>
              <classCode scheme="halDomain" n="chim.mate">Chemical Sciences/Material chemistry</classCode>
              <classCode scheme="halDomain" n="chim.cris">Chemical Sciences/Cristallography</classCode>
              <classCode scheme="halTypology" n="ART">Journal articles</classCode>
              <classCode scheme="halOldTypology" n="ART">Journal articles</classCode>
              <classCode scheme="halTreeTypology" n="ART">Journal articles</classCode>
            </textClass>
            <abstract xml:lang="en">
              <p>The growth of core–shell nanocrystals (NCs) can lead to extended interface disorder due to the intermixing of core and shell materials. Such an issue is particularly important for large single- and multi-shell upconverting NCs, which have been considered as being relatively insusceptible to intermixing. In this work, a robust methodology – based on structure-independent local chemical analyses with nanometer-scale resolution and high-energy synchrotron X-ray powder diffraction – has been used to shed new light on the chemical and structural organization of large single-, double-, and triple-shell upconverting NCs. The experimental results reveal, for the first time, that significant disorder: (i) exists at the interfaces of large (20–50 nm) multi-shell upconverting NCs; (ii) reaches core–shell and shell–shell interfaces, independently of their position within the structure; (iii) can be partially controlled by the shell deposition method; and (iv) leads to the formation of multiple length-scale interfaces depending on the size of the starting seeds, the number and relative thickness of the pre-existing shells in the seeds. It is anticipated that the results will be beneficial in furthering the fundamental understanding of the structure–property relationships of multi-shell upconverting NCs.</p>
            </abstract>
          </profileDesc>
        </biblFull>
      </listBibl>
    </body>
    <back>
      <listOrg type="structures">
        <org type="institution" xml:id="struct-150665" status="VALID">
          <idno type="ISNI">0000 0001 0075 5874</idno>
          <idno type="ROR">https://ror.org/04t3en479</idno>
          <orgName>Karlsruhe Institute of Technology = Karlsruher Institut für Technologie</orgName>
          <orgName type="acronym">KIT</orgName>
          <date type="start">1825-01-01</date>
          <desc>
            <address>
              <addrLine>Campus North, Hermann-von-Helmholtz-Platz 1, 76344 Eggenstein-Leopoldshafen / Campus South, Kaiserstraße 12, 76131 Karlsruhe</addrLine>
              <country key="DE"/>
            </address>
            <ref type="url">https://www.kit.edu/english/</ref>
          </desc>
        </org>
        <org type="researchteam" xml:id="struct-1042408" status="OLD">
          <orgName>Matériaux, Rayonnements, Structure</orgName>
          <orgName type="acronym">NEEL - MRS</orgName>
          <date type="start">2016-01-01</date>
          <date type="end">2019-12-31</date>
          <desc>
            <address>
              <addrLine>Institut NEEL, 25 rue des Martyrs, BP 166,38042 Grenoble cedex 9</addrLine>
              <country key="FR"/>
            </address>
          </desc>
          <listRelation>
            <relation active="#struct-1042377" type="direct"/>
            <relation active="#struct-89889" type="indirect"/>
            <relation name="UPR2940" active="#struct-441569" type="indirect"/>
            <relation active="#struct-445543" type="indirect"/>
          </listRelation>
        </org>
        <org type="regrouplaboratory" xml:id="struct-3392" status="VALID">
          <idno type="IdRef">032927622</idno>
          <orgName>Brookhaven National Laboratory [Upton, NY]</orgName>
          <orgName type="acronym">BNL</orgName>
          <date type="start">1947-01-01</date>
          <desc>
            <address>
              <addrLine>Brookhaven Avenue, Upton, NY 11973</addrLine>
              <country key="US"/>
            </address>
            <ref type="url">http://www.bnl.gov/world/</ref>
          </desc>
          <listRelation>
            <relation active="#struct-301590" type="direct"/>
            <relation active="#struct-303386" type="direct"/>
            <relation active="#struct-361557" type="indirect"/>
            <relation active="#struct-361287" type="direct"/>
          </listRelation>
        </org>
        <org type="laboratory" xml:id="struct-1042377" status="OLD">
          <idno type="IdRef">183998693</idno>
          <idno type="ISNI">0000 0004 0369 268X</idno>
          <idno type="RNSR">200717524X</idno>
          <idno type="ROR">https://ror.org/04dbzz632</idno>
          <orgName>Institut Néel</orgName>
          <orgName type="acronym">NEEL</orgName>
          <date type="start">2016-01-01</date>
          <date type="end">2019-12-31</date>
          <desc>
            <address>
              <addrLine>Institut NEEL, 25 rue des Martyrs, BP 166,38042 Grenoble cedex 9</addrLine>
              <country key="FR"/>
            </address>
            <ref type="url">http://www.neel.cnrs.fr/</ref>
          </desc>
          <listRelation>
            <relation active="#struct-89889" type="direct"/>
            <relation name="UPR2940" active="#struct-441569" type="direct"/>
            <relation active="#struct-445543" type="direct"/>
          </listRelation>
        </org>
        <org type="institution" xml:id="struct-89889" status="OLD">
          <idno type="IdRef">026388804</idno>
          <idno type="ROR">https://ror.org/05sbt2524</idno>
          <orgName>Institut polytechnique de Grenoble - Grenoble Institute of Technology</orgName>
          <orgName type="acronym">Grenoble INP</orgName>
          <date type="start">2007-01-01</date>
          <date type="end">2019-12-31</date>
          <desc>
            <address>
              <addrLine>46 avenue Félix Viallet 38031 Grenoble Cedex 1</addrLine>
              <country key="FR"/>
            </address>
            <ref type="url">http://www.grenoble-inp.fr/</ref>
          </desc>
        </org>
        <org type="regroupinstitution" xml:id="struct-441569" status="VALID">
          <idno type="IdRef">02636817X</idno>
          <idno type="ISNI">0000000122597504</idno>
          <idno type="ROR">https://ror.org/02feahw73</idno>
          <orgName>Centre National de la Recherche Scientifique</orgName>
          <orgName type="acronym">CNRS</orgName>
          <date type="start">1939-10-19</date>
          <desc>
            <address>
              <country key="FR"/>
            </address>
            <ref type="url">https://www.cnrs.fr/</ref>
          </desc>
        </org>
        <org type="institution" xml:id="struct-445543" status="OLD">
          <idno type="IdRef">188399275</idno>
          <idno type="ROR">https://ror.org/02rx3b187</idno>
          <orgName>Université Grenoble Alpes [2016-2019]</orgName>
          <orgName type="acronym">UGA [2016-2019]</orgName>
          <date type="start">2016-01-01</date>
          <date type="end">2019-12-31</date>
          <desc>
            <address>
              <addrLine>38058 Grenoble cedex</addrLine>
              <country key="FR"/>
            </address>
          </desc>
        </org>
        <org type="institution" xml:id="struct-301590" status="VALID">
          <idno type="ROR">https://ror.org/04nza6677</idno>
          <orgName>UT-Battelle, LLC</orgName>
          <date type="start">2000-01-01</date>
          <desc>
            <address>
              <addrLine>1201 Oak Ridge Turnpike, Suite 100, Oak Ridge, TN 37830</addrLine>
              <country key="US"/>
            </address>
            <ref type="url">https://www.ut-battelle.org</ref>
          </desc>
        </org>
        <org type="institution" xml:id="struct-303386" status="VALID">
          <idno type="ISNI">0000 0001 2216 9681</idno>
          <idno type="ROR">https://ror.org/05qghxh33</idno>
          <orgName>Stony Brook University [SUNY]</orgName>
          <orgName type="acronym">SBU</orgName>
          <desc>
            <address>
              <addrLine>100 Nicolls Road, Stony Brook, NY 11794</addrLine>
              <country key="US"/>
            </address>
            <ref type="url">http://www.stonybrook.edu</ref>
          </desc>
          <listRelation>
            <relation active="#struct-361557" type="direct"/>
          </listRelation>
        </org>
        <org type="regroupinstitution" xml:id="struct-361557" status="VALID">
          <idno type="IdRef">026425157</idno>
          <idno type="ROR">https://ror.org/01q1z8k08</idno>
          <orgName>State University of New York</orgName>
          <orgName type="acronym">SUNY</orgName>
          <desc>
            <address>
              <country key="US"/>
            </address>
            <ref type="url">http://www.suny.edu/</ref>
          </desc>
        </org>
        <org type="institution" xml:id="struct-361287" status="VALID">
          <idno type="IdRef">026376903</idno>
          <orgName>U.S. Department of Energy [Washington]</orgName>
          <orgName type="acronym">DOE</orgName>
          <desc>
            <address>
              <addrLine>1000 Independence Ave. SW, Washington DC 20585</addrLine>
              <country key="US"/>
            </address>
            <ref type="url">https://www.energy.gov/</ref>
          </desc>
        </org>
      </listOrg>
    </back>
  </text>
</TEI>