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            <title xml:lang="en">Rydberg Tagging of Spin-Polarized Hydrogen Atoms</title>
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                <forename type="first">Bernadette</forename>
                <surname>Broderick</surname>
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                <forename type="first">Michael</forename>
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                <forename type="first">Baptiste</forename>
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                <forename type="first">Arthur G.</forename>
                <surname>Suits</surname>
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            <idno type="halRefHtml">&lt;i&gt;Atomic and Molecular Interactions, Gordon Research Conference&lt;/i&gt;, Jul 2012, Stonehill College, MA, United States</idno>
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                <title xml:lang="en">Rydberg Tagging of Spin-Polarized Hydrogen Atoms</title>
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                    <surname>Broderick</surname>
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              <p>While the production of spin-polarized hydrogen atoms in photodissociation was predicted over thirty years ago, schemes to quantify it have proved elusive with only a few examples in the literature. The most important experimental difficulty is to resolve the fine structure splitting in the H atom 2p level that is generally far smaller than the associated Doppler width of any transition of interest. Here we show a novel methodology for direct detection of spin-polarized hydrogen atoms with high velocity resolution, which is achieved by a simple modification of the widely used Hydrogen Rydberg time-of-flight technique. This provides a general probe of multi-surface nonadiabatic dynamics, sensitive to coherent effects in dissociation along multiple paths, and applicable to a wide range of polyatomic systems. </p>
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