Coherent vibrational climbing in carboxy-hemoglobin
Résumé
We demonstrate vibrational climbing up to level v=6 in carboxyhemoglobin by use of intense negatively-chirped infrared pulses. This technique gave new spectroscopic insight into carboxy-hemoglobin, such as transition frequencies and dephasing times up to the v=6 to v=7 vibrational transition.