Investigation of $q$-dependent dynamical heterogeneity in a colloidal gel by x-ray photon correlation spectroscopy - Archive ouverte HAL
Article Dans Une Revue Physical Review E : Statistical, Nonlinear, and Soft Matter Physics Année : 2007

Investigation of $q$-dependent dynamical heterogeneity in a colloidal gel by x-ray photon correlation spectroscopy

Résumé

We use time-resolved X-Photon Correlation Spectroscopy to investigate the slow dynamics of colloidal gels made of moderately attractive carbon black particles. We show that the slow dynamics is temporally heterogeneous and quantify its fluctuations by measuring the variance $\chi$ of the instantaneous intensity correlation function. The amplitude of dynamical fluctuations has a non-monotonic dependence on scattering vector $q$, in stark contrast with recent experiments on strongly attractive colloidal gels [Duri and Cipelletti, \textit{Europhys. Lett.} \textbf{76}, 972 (2006)]. We propose a simple scaling argument for the $q$-dependence of fluctuations in glassy systems that rationalizes these findings.
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Dates et versions

hal-00133792 , version 1 (27-02-2007)
hal-00133792 , version 2 (11-04-2007)
hal-00133792 , version 3 (16-11-2007)

Identifiants

Citer

Veronique Trappe, Estelle Pitard, Laurence Ramos, Aymeric Robert, Hugo Bissig, et al.. Investigation of $q$-dependent dynamical heterogeneity in a colloidal gel by x-ray photon correlation spectroscopy. Physical Review E : Statistical, Nonlinear, and Soft Matter Physics, 2007, 76 (5), pp.051404. ⟨10.1103/PhysRevE.76.051404⟩. ⟨hal-00133792v3⟩
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